emep:page1:pm_underestimation

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emep:page1:pm_underestimation [2011-08-24 13:09:38]
hildef
emep:page1:pm_underestimation [2022-05-31 09:29:32] (current)
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 Participants: Participants:
-DS,ST,DS,JEJ,BMS,ACB,MG,HF,PW+DS,ST,JEJ,BMS,ACB,MG,HF,PW,MS
  
 Possible reasons: Possible reasons:
 + 
  * pH dependency of SO2 ox rate \\   * pH dependency of SO2 ox rate \\ 
  * wet scavenging (in ice, scavenging rates ...)\\   * wet scavenging (in ice, scavenging rates ...)\\ 
- * emission heights (probably not important)\\  + * emission heights:\\  
- * Size of vertical layers\\  +DS:I have started this, testing different plume-rise 
- * BIC for aerosols\\  +formula together with the IIASA . Peter contributed with a subroutine to 
- * Wood burning emissions\\ +spread the emissions into flexible vertical layers also. Should all be 
 +ready soon-ish, but probably won't change things very much as you say. (probably not important)\\   
 + 
 + * Size of vertical layers, boundary layer mixing \\  
 + * Secondary Organic Aerosol contribution\\ 
 + * Agricultural and Industrial dust in windy, dry conditions \\  
 + * BIC for aerosols, dust in southern Europe\\  
 + * Wood burning emissions underestimated:Robert is doing  a lot with Hugo as we speak, but the problem is with the "official" emissions. We can't change them, even 
 +when we know they are wrong. \\ 
 +We could change the time-series though, using a "degree-day" approach as 
 +Betrand used. That would be good, but requires some testing. I think 
 +that SNAP-2 in general should have this, and wood-burning especially, 
 +but I also suspect that wood-burning starts at a lower temperature than 
 +Betrand's 20C degree days. \\   
 +* Station representativity for some specific sites (Susceptibility to inversion situations in winter?)\\ 
 +* Kz, Hmix - currently our minimum mixing height is in the 2nd layer 
 +(k=19). I have some test versions which allow very shallow mixing 
 +heights. These cause a slight increase in surface PM, and are 
 +scientifically ok I think. I can commit next week if all looks well. \\  
 +(What I am less sure about is what we should do for Kz above Hmix. Now 
 +we have zero, earlier we used critical Richardson numbers, etc. Seems 
 +better to use the latter.) \\  
 + 
 +* I suggested some ideas for David H. here to work with, but that seems 
 +to be progressing slowly. I'll check again on this next week. \\  
 + 
 +* Ammonium nitrate formation \\ 
 +* Emission seasonality for SO2 missing\\ 
 + 
 +Which Analysis : 
 + 
 +* Separate discussion by aerosol component\\ 
 +* AMS measurements EUSAAR ?\\ 
 +* Caliop extinction profiles for European subregions become available shortly, extinction profile in model needed, \\ 
 +* EUCAARI aircraft measurements?\\ 
 +* Seasonal and spatial bias analysis \\  
 +** When do we underestimate?? It would be good to use time to figure out 
 +if we can see patterns in the days when we underestimate compared to 
 +when we don't. Is it on very cold days, or generally for example?  Which 
 +compounds cause most of the problem? Might give a clue on whether it is 
 +meteorology of chemistry. \\  
 + 
 +===== Minutes ===== 
 + 
 + * [[emep:page2:Minutes|Minutes 26.08.2011]]
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