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aerocom:organics [2012-07-04 15:35:54] mariak@chemistry.uoc.gr |
aerocom:organics [2022-05-31 09:29:31] (current) |
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| + | ATTENTION - THIS WIKI PAGE IS NO LONGER UPDATED - PLEASE GO TO [[http:// | ||
| + | |||
| ====== Organic aerosol documentation ====== | ====== Organic aerosol documentation ====== | ||
| Please e-mail Kostas Tsigaridis (kostas.tsigaridis@columbia.edu) in case you make changes in this page. | Please e-mail Kostas Tsigaridis (kostas.tsigaridis@columbia.edu) in case you make changes in this page. | ||
| + | |||
| + | **Abbreviations used in emissions** | ||
| + | |||
| + | * CIRCE: Climate Change and Impact Research: the Mediterranean Environment (http:// | ||
| + | * CMIP5: Coupled Model Intercomparison Project phase 5 (http:// | ||
| + | * GEIA: Global Emissions Inventory Activity (http:// | ||
| + | * GFED: Global Fire Emissions Database (van der Werf et al., 2003). | ||
| + | * GFED2: Global Fire Emissions Database, version 2 (van der Werf et al., 2006). | ||
| + | * GFED3: Global Fire Emissions Database, version 3 (van der Werf et al., 2010). | ||
| + | * MEGAN: Model of Emissions of Gases and Aerosols from Nature (Guenther et al., 2006). | ||
| ===== BCC ===== | ===== BCC ===== | ||
| Line 8: | Line 20: | ||
| **OA representation** | **OA representation** | ||
| - | * 12 primary | + | * 12 OA tracers |
| - | * no SOA | + | * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA |
| - | * OM/OC: 1.6 | + | * OM/OC: 1.4 |
| **Primary OA Emissions** | **Primary OA Emissions** | ||
| * Fossil fuel and biofuel: Bond et al. (2004), year 2000 | * Fossil fuel and biofuel: Bond et al. (2004), year 2000 | ||
| * Biomass burning: GFED, year 2000 | * Biomass burning: GFED, year 2000 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * None | + | * Monoterpenes: |
| ===== CAM4-Oslo ===== | ===== CAM4-Oslo ===== | ||
| Line 22: | Line 34: | ||
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| - | * 38.5 Tg/a from terpenes emissions based on Dentener er al. (2006) distribution, | + | * 37.5 Tg/a from terpenes emissions based on Dentener er al. (2006) distribution, |
| * OM/OC: 1.4 for fossil fuel, 2.6 for biomass burning | * OM/OC: 1.4 for fossil fuel, 2.6 for biomass burning | ||
| **Primary OA emissions** | **Primary OA emissions** | ||
| - | * Fossil fuel and biofuel: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Fossil fuel and biofuel: AeroCom |
| * Primary marine OA: Spracklen et al. (2008), year 2006 | * Primary marine OA: Spracklen et al. (2008), year 2006 | ||
| - | * Biomass burning: AeroCom hindcast inventory | + | * Biomass burning: AeroCom |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Monoterpenes: | * Monoterpenes: | ||
| Line 37: | Line 49: | ||
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| * Prescribed mass yields for the 5 SOA precursor categories, (6.0, 37.5, 22.5, 7.5, and 7.5% respectively) which then reversibly partition to the aerosol phase | * Prescribed mass yields for the 5 SOA precursor categories, (6.0, 37.5, 22.5, 7.5, and 7.5% respectively) which then reversibly partition to the aerosol phase | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| Line 44: | Line 56: | ||
| * Biomass burning: CMIP5, year 2000 | * Biomass burning: CMIP5, year 2000 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Isoprene, terpenes, aromatics, higher molecular weight alkanes and alkenes: Horowitz | + | * Isoprene, terpenes, aromatics, higher molecular weight alkanes and alkenes. Emissions files produced for MOZART-4 (Emmons |
| ===== CanAM-PAM ===== | ===== CanAM-PAM ===== | ||
| Line 51: | Line 63: | ||
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Fossil fuel and biofuel: AeroCom |
| - | * Biomass burning: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Biomass burning: AeroCom |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Monoterpenes | * Monoterpenes | ||
| Line 63: | Line 75: | ||
| ECHAM5-HAMMOZ.A2.HCA-0 | ECHAM5-HAMMOZ.A2.HCA-0 | ||
| + | |||
| + | **OA representation** | ||
| + | * 4 OA tracers | ||
| + | * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | ||
| + | * OM/OC: 1.4 | ||
| + | |||
| + | **primary OA emissions** | ||
| + | * Fossil fuel and biofuel: Diehl et al. (2012), years 1980-2005 | ||
| + | * Biomass burning: RETRO (M. Schultz) for 1980-2000, GFED2 for 2001-2005 | ||
| + | |||
| + | **SOA precursor emissions** | ||
| + | * Monoterpenes: | ||
| ===== ECHAM5-SALSA ===== | ===== ECHAM5-SALSA ===== | ||
| Line 69: | Line 93: | ||
| **OA representation** | **OA representation** | ||
| - | * 11 primary | + | * 11 OA tracers |
| * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: Bond et al., (2004), year 2000 | + | * Fossil fuel and biofuel: Bond et al. (2004), year 2000 |
| * Biomass burning: GFED, year 2000 | * Biomass burning: GFED, year 2000 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| Line 83: | Line 107: | ||
| **OA representation** | **OA representation** | ||
| - | * 2 primary | + | * 2 OA tracers |
| * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | * 15% yield from terpenes emissions (Dentener et al., 2006) included in primary OA | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: Dentener et al., (2006), year 2000 | + | * Fossil fuel and biofuel: Dentener et al. (2006), year 2000 |
| - | * Biomass burning: Dentener et al., (2006), year 2000 | + | * Biomass burning: Dentener et al. (2006), year 2000 |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Monoterpenes | * Monoterpenes | ||
| Line 97: | Line 121: | ||
| **OA representation** | **OA representation** | ||
| - | * 5 primary | + | * 5 OA tracers |
| * 2-product model | * 2-product model | ||
| * OM/OC: 2.1 | * OM/OC: 2.1 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: Bond et al., (2007), year 2000 | + | * Fossil fuel and biofuel: Bond et al. (2007), year 2000 |
| * Biomass burning: GFED2, year 2006 | * Biomass burning: GFED2, year 2006 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| Line 111: | Line 135: | ||
| **OA representation** | **OA representation** | ||
| - | * 24 primary | + | * 24 OA tracers |
| * 2-product model combined with aging and condensation | * 2-product model combined with aging and condensation | ||
| * OM/OC: 2.1 | * OM/OC: 2.1 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: Bond et al., (2007), year 2000 | + | * Fossil fuel and biofuel: Bond et al. (2007), year 2000 |
| * Biomass burning: GFED2, year 2006 | * Biomass burning: GFED2, year 2006 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| Line 127: | Line 151: | ||
| **OA representation** | **OA representation** | ||
| - | * 26 primary | + | * 26 OA tracers |
| * Volatility basis set | * Volatility basis set | ||
| * OM/OC: 1.8 | * OM/OC: 1.8 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: Bond et al., (2004), year 2000 | + | * Fossil fuel and biofuel: Bond et al. (2004), year 2000 |
| * Biomass burning: GFED2, year 2005 | * Biomass burning: GFED2, year 2005 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Isoprene, monoterpenes, | * Isoprene, monoterpenes, | ||
| - | * Aromatics (VOC's with C*<1e6 μg/m³): Farina et al., (2010), year 1999 | + | * Aromatics (VOC's with C*<1e6 μg/m³): Farina et al. (2010), year 1999 |
| - | * Alkanes, alkenes (VOC's with C*<1e6 μg/m³): Farina et al., (2010), year 1999 | + | * Alkanes, alkenes (VOC's with C*<1e6 μg/m³): Farina et al. (2010), year 1999 |
| | | ||
| ===== GISS-MATRIX ===== | ===== GISS-MATRIX ===== | ||
| Line 143: | Line 167: | ||
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| - | * 10% yield from monoterpenes emissions | + | * 10% yield from monoterpenes emissions, included in primary OA |
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| Line 150: | Line 174: | ||
| * Biomass burning: GFED3, years 2006-2008 | * Biomass burning: GFED3, years 2006-2008 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Monoterpenes | + | * Monoterpenes: Lathière et al. (2005) |
| - | ===== GISS-modelE-G/ | + | ===== GISS-modelE ===== |
| GISS-modelE.A2.CTRL/ | GISS-modelE.A2.CTRL/ | ||
| **OA representation** | **OA representation** | ||
| - | * 9 primary | + | * 9 OA tracers |
| * 2-product model | * 2-product model | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| * Fossil fuel and biofuel: CMIP5 RCP4.5, years 2000-2008 | * Fossil fuel and biofuel: CMIP5 RCP4.5, years 2000-2008 | ||
| - | * Biomass burning: GFED3 (G)/CMIP5 RCP4.5 (I), years 2000-2008 | + | * Biomass burning: GFED3 (CTRL)/CMIP5 RCP4.5 (HCA-IPCC), years 2000-2008 |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Isoprene: online (Guenther et al., 1995), years 2000-2008 | * Isoprene: online (Guenther et al., 1995), years 2000-2008 | ||
| - | * α-pinene: | + | * α-pinene: |
| ===== GISS-TOMAS ===== | ===== GISS-TOMAS ===== | ||
| Line 172: | Line 196: | ||
| **OA representation** | **OA representation** | ||
| - | * 24 primary | + | * 24 OA tracers |
| * A generic SOA precursor (GEIA) representing all SOA precursor gases is emitted and forms non-volatile SOA (included in primary OA) with a first order loss rate of 12 hours | * A generic SOA precursor (GEIA) representing all SOA precursor gases is emitted and forms non-volatile SOA (included in primary OA) with a first order loss rate of 12 hours | ||
| * OM/OC: 1.8 | * OM/OC: 1.8 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Fossil fuel and biofuel: AeroCom |
| - | * Biomass burning: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Biomass burning: AeroCom |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Terpenes | + | * Terpenes: GEIA, year 1990 |
| - | ===== GLOMAPbin/ | + | ===== GLOMAP |
| GLOMAPbin1pt1.A2.CTRL/ | GLOMAPbin1pt1.A2.CTRL/ | ||
| **OA representation** | **OA representation** | ||
| - | * 40 (bin), 5 (mode) | + | * 40 (bin), 5 (mode) OA tracers |
| * α-pinene and all oxidants with 13% non-volatile SOA (included in primary OA) | * α-pinene and all oxidants with 13% non-volatile SOA (included in primary OA) | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: Dentener et al., (2006), year 2000 | + | * Fossil fuel and biofuel: Dentener et al. (2006), year 2000 |
| - | * Biomass burning: Dentener et al., (2006), year 2000 | + | * Biomass burning: Dentener et al. (2006), year 2000 |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * α-pinene | + | * α-pinene: GEIA, year 1990 |
| ===== GMI ===== | ===== GMI ===== | ||
| Line 200: | Line 224: | ||
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| - | * 10% yield from monoterpenes emissions from GEIA (Guenther et al., 1995), included in primary OA | + | * 10% yield from monoterpenes emissions from GEIA, included in primary OA |
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| Line 207: | Line 231: | ||
| * Biomass burning: CMIP5, year 2000 | * Biomass burning: CMIP5, year 2000 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Monoterpenes | + | * Monoterpenes: GEIA, year 1990 |
| ===== GOCART ===== | ===== GOCART ===== | ||
| Line 214: | Line 238: | ||
| **OA representation** | **OA representation** | ||
| - | * 2 primary | + | * 2 OA tracers |
| * 10% yield from monoterpenes emissions (GEIA), included in primary OA | * 10% yield from monoterpenes emissions (GEIA), included in primary OA | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Fossil fuel and biofuel: AeroCom |
| - | * Biomass burning: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Biomass burning: AeroCom |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Monoterpenes | + | * Monoterpenes: GEIA, year 1990 |
| ===== HadGEM2 ===== | ===== HadGEM2 ===== | ||
| Line 228: | Line 252: | ||
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| * Fixed 3D monthly climatology obtained from STOCHEM (Derwent et al., 2003) | * Fixed 3D monthly climatology obtained from STOCHEM (Derwent et al., 2003) | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| Line 237: | Line 261: | ||
| * Terpenes: GEIA, year 1990 | * Terpenes: GEIA, year 1990 | ||
| - | ===== IMAGES ===== | + | ===== IMPACT ===== |
| - | + | ||
| - | **OA representation** | + | |
| - | * 26 primary OA tracers | + | |
| - | * 2-product model | + | |
| - | * OM/OC: varying | + | |
| - | **primary OA emissions** | + | |
| - | * Fossil fuel and biofuel: Bond et al., (2004), year 2000 | + | |
| - | * Biomass burning: GFED2, year 2000 | + | |
| - | **SOA precursor emissions** | + | |
| - | * Isoprene: MEGAN, year 2006 | + | |
| - | * α-pinene, sesquiterpenes: | + | |
| - | * Benzene, toluene, xylene: RETRO, year 2000 | + | |
| - | + | ||
| - | ===== IMPACT-A/ | + | |
| - | IMPACT-A.A2.CTRL/ | + | IMPACT-Umich.A2.CTRL |
| ===== LMDz-INCA ===== | ===== LMDz-INCA ===== | ||
| - | LSCE-vRV.A2.CTRL | + | INCA.A2.RAD-CTRL |
| **OA representation** | **OA representation** | ||
| - | * 3 primary | + | * 3 OA tracers |
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| Line 268: | Line 278: | ||
| **OA representation** | **OA representation** | ||
| - | * 24 primary | + | * 24 OA tracers |
| * 2-product model | * 2-product model | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Fossil fuel and biofuel: AeroCom |
| - | * Biomass burning: AeroCom hindcast inventory, Diehl et al., (2008), year 2006 | + | * Biomass burning: AeroCom |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Isoprene: MEGAN, year 2006 | * Isoprene: MEGAN, year 2006 | ||
| Line 281: | Line 291: | ||
| ===== OsloCTM2 ===== | ===== OsloCTM2 ===== | ||
| - | OsloCTM2.A2.CTRL | + | OsloCTM2-v2.A2.CTRL |
| **OA representation** | **OA representation** | ||
| - | * 62 primary | + | * 62 OA tracers |
| * 2-product model | * 2-product model | ||
| * OM/OC: 1.6 for fossil fuel and 2.6 for biomass burning | * OM/OC: 1.6 for fossil fuel and 2.6 for biomass burning | ||
| Line 292: | Line 302: | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| * Isoprene: POET scaled to 220 Tg/a, year 2000 | * Isoprene: POET scaled to 220 Tg/a, year 2000 | ||
| - | * 5 classes of terpenoid compounds: Griffin et al., (1999b), GEIA, year 1990 | + | * 5 classes of terpenoid compounds: Griffin et al. (1999b), GEIA, year 1990 |
| * 2 classes of aromatics: CMIP5, year 2000 | * 2 classes of aromatics: CMIP5, year 2000 | ||
| Line 300: | Line 310: | ||
| **OA representation** | **OA representation** | ||
| - | * 2 primary | + | * 2 OA tracers |
| - | * 9.225% yield of non-volatile SOA (Griffin et al., 1999a, | + | * 9.225% yield of non-volatile SOA (Griffin et al., 1999a, |
| * OM/OC: 1.6 for fossil fuel and biofuel, 2.6 for other | * OM/OC: 1.6 for fossil fuel and biofuel, 2.6 for other | ||
| **primary OA emissions** | **primary OA emissions** | ||
| - | * Fossil fuel and biofuel: | + | * Fossil fuel and biofuel: |
| - | * Biomass burning: | + | * Biomass burning: |
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Monoterpenes | + | * Monoterpenes: GEIA, year 1990 |
| - | ===== TM4-ECPL-C/ | + | ===== TM4-ECPL ===== |
| TM4-ECPL-C.A2.CTRL | TM4-ECPL-C.A2.CTRL | ||
| + | |||
| TM4-ECPL-F.A2.CTRL | TM4-ECPL-F.A2.CTRL | ||
| + | |||
| TM4-ECPL-FNP.A2.CTRL | TM4-ECPL-FNP.A2.CTRL | ||
| **OA representation** | **OA representation** | ||
| - | * 20 primary | + | * 20 OA tracers (24 for FNP version) |
| * 2-product model | * 2-product model | ||
| * OM/OC: varying | * OM/OC: varying | ||
| Line 332: | Line 344: | ||
| **OA representation** | **OA representation** | ||
| - | * 4 primary | + | * 4 OA tracers |
| * 15% yield from terpenes emissions (Dentener et al., 2006), included in primary OA | * 15% yield from terpenes emissions (Dentener et al., 2006), included in primary OA | ||
| * OM/OC: 1.4 | * OM/OC: 1.4 | ||
| Line 339: | Line 351: | ||
| * Biomass burning: CMIP5 RCP4.5, years 2000-2009 | * Biomass burning: CMIP5 RCP4.5, years 2000-2009 | ||
| **SOA precursor emissions** | **SOA precursor emissions** | ||
| - | * Monoterpenes | + | * Monoterpenes: GEIA, year 1990 |